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- W1526492536 abstract "As a key factor leading to the pressure-dependent R1-line-shift reversal and R1-state lifetime, at 10 K, the pressure-dependent variation of mixing-degree of |t22(3T1)e4T2 and |t232E base-wavefunctions in the wavefunction of R1 state of LLGG:Cr3+ has been calculated and analyzed. From this, the physical origin of the pressure-dependent R1-line-shift reversal has been revealed. Furthermore, by using the pressure-dependent values of the sum of all square mixing-coefficients of |t22(3T1)e4T2 in the wavefunction of R1 state, the lifetimes of R1 state of LLGG:Cr3+ at various pressures have been calculated, which are in good agreement with observed results. The quantum anticrossing effect between t232E and t22(3T1)e4T2 levels due to both spin-orbital interaction and electron-phonon interaction is remarkable, which is related to the admixture of |t22(3T1)e4T2 and |t232E as well as the low–high crystal-field transition." @default.
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- W1526492536 date "2006-06-01" @default.
- W1526492536 modified "2023-09-27" @default.
- W1526492536 title "Pressure-Dependent Base-Wavefunction Admixture and Lifetime of R 1 State of La 3 Lu 2 Ga 3 O 12 :Cr 3+" @default.
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- W1526492536 doi "https://doi.org/10.1088/0253-6102/45/6/035" @default.
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