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- W1527984967 abstract "Potential transients are obtained by using “Padé approximants” (an accurate approximation procedure valid globally — not just perturbatively) for all amplitudes of concentration polarization and current densities. This is done for several mechanistic schemes under constant current conditions. We invert the non-linear current-potential relationship in the form (using the Lagrange or the Ramanujan method) of power series appropriate to the two extremes, namely near reversible and near irreversible. Transforming both into the Pad́e expressions, we construct the potential-time profile by retaining whichever is the more accurate of the two. The effectiveness of this method is demonstrated through illustrations which include couplings of homogeneous chemical reactions to the electron-transfer step." @default.
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- W1527984967 date "1990-01-01" @default.
- W1527984967 modified "2023-09-27" @default.
- W1527984967 title "Padé approach to potential transients" @default.
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- W1527984967 doi "https://doi.org/10.1016/0022-0728(90)85089-n" @default.
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