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- W1533131838 abstract "The effects of metal species in an Fe-based catalyst on structural properties were investigated through the synthesis of Fe-based catalysts containing various metal species such, as Mn, Zr, and Ce. The addition of the metal species to the Fe-based catalyst resulted in high dispersions of the Fe species and high surface areas due to the formation of mesoporous voids about 2–4 nm surrounded by the catalyst particles. The metal-added Fe-based catalysts were employed together with Co-loaded beta zeolite for the synthesis of hydrocarbons from syngas with a lower H 2 /CO ratio of 1 than the stoichiometric H 2 /CO ratio of 2 for the Fischer-Tropsch synthesis (FTS). Among the catalysts, the Mn-added Fe-based catalyst exhibited a high activity for the water-gas shift (WGS) reaction with a comparative durability, leading to the enhancement of the CO hydrogenation in the FTS in comparison with Co-loaded beta zeolite alone. Furthermore, the loading of Pd on the Mn-added Fe-based catalyst enhanced the catalytic durability due to the hydrogenation of carbonaceous species by the hydrogen activated over Pd." @default.
- W1533131838 created "2016-06-24" @default.
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- W1533131838 date "2015-01-01" @default.
- W1533131838 modified "2023-09-25" @default.
- W1533131838 title "Synthesis of Hydrocarbons from H2-Deficient Syngas in Fischer-Tropsch Synthesis over Co-Based Catalyst Coupled with Fe-Based Catalyst as Water-Gas Shift Reaction" @default.
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- W1533131838 doi "https://doi.org/10.1155/2015/268121" @default.
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