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• W1533152044 abstract "The replacement of one C-atom by an N-atom in C60 leads to changes of its geometrical and electronic properties. The resulting heterofullerene radical forms (C59N)2 dimers in the bulk. We have used high resolution electron energy loss spectroscopy (HREELS) to investigate the vibrational and electronic excitations of this novel modified fullerene which we deposited as a multilayer film on single crystal graphite C(0001). The frequencies of the vibrational modes are generally close to those of C60, except for two new modes which can be attributed to the dimer: an intra-dimer vibration at around 18 meV and a dipole-active mode at 104 meV. The electronic excitation spectrum is also similar to that of C60 regarding the interband transitions, despite a broadening due to the lower symmetry in (C59N)2. However, in contrast to C60, the first excitonic excitations seen at 1.55 and 1.75 eV are now dipole allowed." @default.
• W1533152044 created "2016-06-24" @default.
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• W1533152044 date "2000-01-01" @default.
• W1533152044 modified "2023-09-23" @default.
• W1533152044 title "HREELS investigations of adsorbed (C[sub 59]N)[sub 2]" @default.
• W1533152044 doi "https://doi.org/10.1063/1.1342478" @default.
• W1533152044 hasPublicationYear "2000" @default.
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