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• W1538182566 abstract "The translational anisotropy and angular momentum polarization of the O(2)(a (1)Delta(g),v = 0;J = 15-27) molecular photofragment produced from the UV photodissociation of O(3) in the range from 270 to 300 nm have been determined using resonance-enhanced multiphoton ionization in conjunction with time-of-flight mass spectrometry. At the shortest photolysis wavelengths used, the fragments exhibit the anisotropic vector correlations expected from a prompt dissociation via the (1)B(2) <--(1)A(1) transition. Deviations from this behavior are observed at longer photolysis wavelengths with, in particular, the angular momentum orientation showing a significant reduction in magnitude. This indicates that the dissociation can no longer be described by a purely impulsive model and a change in geometry of the dissociating molecule is implied. This observation is substantiated by the variation of the translational anisotropy with photolysis wavelength. We also observe that the bipolar moments describing the angular momentum polarization of the odd J states probed are consistently lower in magnitude than those of the even J states and that this variation is observed for all photolysis wavelengths." @default.
• W1538182566 created "2016-06-24" @default.
• W1538182566 creator A5035516379 @default.
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• W1538182566 date "2005-06-22" @default.
• W1538182566 modified "2023-09-24" @default.
• W1538182566 title "Photolysis wavelength dependence of the translational anisotropy and the angular momentum polarization of O2(aΔg1) formed from the UV photodissociation of O3" @default.
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• W1538182566 doi "https://doi.org/10.1063/1.1944719" @default.
• W1538182566 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16035771" @default.
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