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• W1539556076 abstract "Being a challenging and promising field from both academic and industrial perspective, combination of biocatalysis with chemocatalysis or “classic chemical” processes towards one-pot processes has emerged in recent years tremendously. A representative advantage of such processes is the avoidance of time- and capacity consuming and waste producing work-up steps which are required when conducting reactions in a sequential fashion with intermediate isolations and purifications. Furthermore, solvent usage can be dramatically shortened and also space-time yields can be significantly improved. As a key issue for the set-up of such one-pot processes – independent of the concept which is applied – one can regard to achieve compatibility of the individual steps with each other. So far two types of concepts of chemoenzymatic one-pot processes in terms of reaction types being involved have been mainly studied. The first concept is based on an isomerization of a substrate, which is catalyzed by means of a chemocatalyst, and its combination with an in situ enzymatic transformation of one of the isomers. As isomers mostly racemic mixtures of enantiomers are used, which then leads to dynamic kinetic resolution processes. The second concept is based on a combination of a substrate synthesis (not formed by an isomerization process) in an initial step, followed by a subsequent transformation of the substrate. In these processes, the biotransformation can be integrated as initial or as subsequent step dependent on the desired product and reaction sequence. For these concepts, a range of synthetic examples have now been developed, which are summarized in this review." @default.
• W1539556076 created "2016-06-24" @default.
• W1539556076 creator A5043185127 @default.
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• W1539556076 date "2014-06-27" @default.
• W1539556076 modified "2023-10-05" @default.
• W1539556076 title "Chemoenzymatic Multistep One‐Pot Processes" @default.
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• W1539556076 doi "https://doi.org/10.1002/9783527682492.ch19" @default.
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