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- W1539978411 abstract "Structure formation and self-assembly of physisorbed and chemisorbed organic monolayers will be describedon electrified solid–liquid interfaces employing in-situ scanning tunneling microscopy (STM) and surface-enhancedinfrared spectroscopy (SEIRAS) in combination with electrochemical techniques. We present first a casestudy on self-assembly by directional hydrogen bonding and its interplay with the electrode potential choosingaromatic carboxylic acids, with an emphasis on 1,3,5-benzene-tricarboxylic acid (TMA). Structure and electricalcharacteristics of chemisorbed organic monolayers involving the formation of covalent bonds with the substratesurface will be discussed for a series of 4-methyl-4′-(n-mercaptoalkyl)biphenylson Au(111) electrodes. In an attempt to explore single molecule properties, such as charge transport andredox-mediated tunneling, we subsequently introduce an STM-based technique to construct symmetric and asymmetricmetal/(single) molecule/metal junctions. Employing α,ω-alkanedithiols and redox-active derivatives of viologens we demonstratenovel transport and single molecule electrochemical studies, which bear unique novel perspectives for fundamentalas well as applied investigations." @default.
- W1539978411 created "2016-06-24" @default.
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- W1539978411 date "2008-01-01" @default.
- W1539978411 modified "2023-10-17" @default.
- W1539978411 title "From Self-Assembly to Charge Transport with Single Molecules – An Electrochemical Approach" @default.
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