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- W1542101124 abstract "Abstract The steam reforming of four bio-oil model compounds (acetic acid, ethanol, acetone and phenol) was investigated over Ni-based catalysts supported on Al 2 O 3 modified by Mg, Ce or Co in this paper. The activation process can improve the catalytic activity with the change of high-valence Ni (Ni 2 O 3 , NiO) to low-valence Ni (Ni, NiO). Among these catalysts after activation, the Ce-Ni/Co catalyst showed the best catalytic activity for the steam reforming of all the four model compounds. After long-term experiment at 700 °C and the S/C ratio of 9, the Ce-Ni/Co catalyst still maintained excellent stability for the steam reforming of the simulated bio-oil (mixed by the four compounds with the equal masses). With CaO calcinated from calcium acetate as CO 2 sorbent, the catalytic steam reforming experiment combined with continuous in situ CO 2 adsorption was performed. With the comparison of the case without the adding of CO 2 sorbent, the hydrogen concentration was dramatically improved from 74.8% to 92.3%, with the CO 2 concentration obviously decreased from 19.90% to 1.88%." @default.
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- W1542101124 date "2015-05-01" @default.
- W1542101124 modified "2023-10-16" @default.
- W1542101124 title "Hydrogen production via steam reforming of bio-oil model compounds over supported nickel catalysts" @default.
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- W1542101124 doi "https://doi.org/10.1016/s2095-4956(15)60315-1" @default.
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