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- W1544179619 abstract "Ni and/or Rh based catalysts (ex-HT) derived by hydrotalcite precursor are considered to be effective catalysts in the catalytic partial oxidation (CPO) reaction. This chapter discusses new stable ex-HT catalysts prepared by inserting silicate instead of CO32- anions in the interlayer. The amount of silicates is not limited by the charge balance of the cations, because, an excess of silicates leads to the formation of polysilicate anions. The insertion of silicates affects the structure of the calcined samples, because, unlike CO32-, the silicates remain in the structure and contribute to the formation of the final catalysts. Catalysts with innovative structure are obtained by HT precursor prepared using silicate as interlayer anion. The calcined catalysts showed two phases—a mixed oxide type structure and a new M-silicate structure, where the cations of the active metal are partially soluted. The Rh catalyst prepared by HT silicate was more active and selective than the one prepared by CO32-." @default.
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- W1544179619 date "2004-01-01" @default.
- W1544179619 modified "2023-10-14" @default.
- W1544179619 title "New catalysts for the syngas production obtained by hydrotalcite type precursor containing silicate" @default.
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- W1544179619 doi "https://doi.org/10.1016/s0167-2991(04)80053-3" @default.
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