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• W1547185855 abstract "A detailed chemically reacting flow model was developed to study the full-fledged combustion of an initially oxide-free boron particle in a quiescent environment of combustion products. In the model, a surface chemistry mechanism previously developed for fluorine-free environments was extended to include fluorine. The effect of fluorine concentration as well as ambient gas temperature and particle size on burning rates was studied under diffusive- and chemical kinetically controlled conditions. In order to determine the dominant surface reactions, a sensitivity analysis was performed. Model results indicate that: (1) the addition of fluorine shifts the main products from B2O3(g) and HOBO(g) to OBF(g) and BF3(g); (2) for ratios of fluorine to oxygen atoms (F/O) less than 1, the kinetically controlled burning rate decreases slightly, while the diffusive-controlled burning rate decreases significantly with increasing F/O ratio; (3) for F/O ratios greater than 1, the kinetically controlled burning rate increases with F/O ratio, while the diffusive-controlled burning rate is insensitive to F/O ratio; and (4) the surface reactions of B2O3(g), O2(g) and F(g) are found to be the rate-controlling surface reactions with the relative importance of these processes dependent on F/O ratio." @default.
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• W1547185855 date "1998-03-01" @default.
• W1547185855 modified "2023-10-15" @default.
• W1547185855 title "Effect of Fluorine on the Combustion of “Clean” Surface Boron Particles" @default.
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• W1547185855 doi "https://doi.org/10.1016/s0010-2180(97)00129-6" @default.
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