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- W1548045457 abstract "The performance of Fe-MFI zeolites in N2O-and O2-mediated conversion of propane to propene and oxygenates has been investigated over a set of calcined and steamed Fe-MFI (Si/Al=12-620) catalysts containing iron originally in the framework, in cationic sites and as oxide-like supported Fe species. All the catalysts exhibited very low activity in oxidation of propane by molecular oxygen, whereas in the propane reaction with nitrous nitrous oxide the propene yield was up to 20%, besides formation of other oxygenates. The results of UV-Vis and EPR spectroscopy and reaction kinetic tests enabled to suggest that very small part of the well-isolated Fe-species is extremely active in propane oxidation by nitrous oxide following the “propane-propanol-propene-propanal-COx” reaction pathway." @default.
- W1548045457 created "2016-06-24" @default.
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- W1548045457 date "2005-01-01" @default.
- W1548045457 modified "2023-10-17" @default.
- W1548045457 title "Occurrence of Fe species in Fe-zeolites active in propane oxidation with N2O to propene and propanal" @default.
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- W1548045457 doi "https://doi.org/10.1016/s0167-2991(05)80563-4" @default.
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