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- W1550207816 abstract "An interpolation procedure is introduced for obtaining the heat of formation of various halide and oxide compounds. From this scheme it becomes possible to derive the energy difference between trivalent and tetravalent rare-earth and actinide metals (with non-bonding f-electrons). As an example, for cerium it is found that this energy separation is about 40kcal/mol, a finding which definitely rules out the promotion model for this metal. For the early actinide metals the metallic bonding contribution due to the itinerant 5f electrons also becomes evident. From the energy differences between different valence states of the f-metals, a rather extensive stability study of various halide and oxide systems can be undertaken. The success of this investigation reinforces the reliability of the derived energy differences between the metallic valence states." @default.
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- W1550207816 date "1978-01-01" @default.
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- W1550207816 title "Energy difference between trivalent and tetravalent metallic cerium and other f-elements" @default.
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