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• W1552904509 abstract "Among quasi-two-dimensional organic conductors, ${(text{BEDT-TTF})}_{2}X$, what form the two column structure of $ensuremath{alpha}$ or $ensuremath{theta}$ is thought to show a charge-ordering insulating state. The ${ensuremath{alpha}}^{ensuremath{'}}$ modification is the other candidate for a charge-ordering state. To determine the existence of a charge-ordering state and electron magnetism in the ${ensuremath{alpha}}^{ensuremath{'}}$ phase, which has a symmetry that differs from that of the $ensuremath{alpha}$ and $ensuremath{theta}$ phases, we utilized $^{13}text{C}text{-NMR}$ to examine ${ensuremath{alpha}}^{ensuremath{'}}text{ensuremath{-}}{(text{BEDT-TTF})}_{2}{text{IBr}}_{2}$ in which one side of the central carbon on the BEDT-TTF molecule is substituted with $^{13}text{C}$ nuclei. We observed changes in its spectrum at 200 K. The angular dependence of the NMR shift at 15 K indicated that the charge-ordering pattern is intracolumn disproportionation and the ratio of charge disproportionation on the spin-poor site and spin-rich sites is almost 1:0. The angle dependence of NMR spectrum at 60 K suggests that the hyperfine coupling tensor in the paramagnetic charge-ordering state is determined not only by the charge density of on-site molecules but also by the contribution of off-site molecules. The change in hyperfine coupling tensor must be taken into account in NMR studies of the paramagnetic CO state." @default.
• W1552904509 created "2016-06-24" @default.
• W1552904509 creator A5021230879 @default.
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• W1552904509 date "2009-10-02" @default.
• W1552904509 modified "2023-09-25" @default.
• W1552904509 title "<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mmultiscripts><mml:mtext>C</mml:mtext><mml:mprescripts /><mml:none /><mml:mrow><mml:mn>13</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math>NMR study on the charge-ordering salt<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mi>α</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mtext>−</mml:mtext><mml:msub><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mrow…" @default.
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• W1552904509 doi "https://doi.org/10.1103/physrevb.80.165103" @default.
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