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- W155389017 abstract "Abstract One approach to photochemistry is to treat it as a generalization of ordinary kinetics with usual transition state theory concepts governing the design of structure-reactivity studies. This will be valid only if the excited state lifetime is long compared to the rate of rovibrational relaxation. The utility of this approach is well illustrated by the discussion of Cr(bipy) 3 3+ reduction from the microsecond lifetime 2 E state. However, recent evidence concerning reactions of Cr(III) complexes suggests that substitution reactions can occur on a time scale competitive with rovibrational relaxation. This leads to the recognition of limits on conventional classification of reaction mechanisms. It is suggested that an appropriate terminology distinguishes a photochemical and photophysical limit." @default.
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- W155389017 date "1980-01-01" @default.
- W155389017 modified "2023-10-16" @default.
- W155389017 title "PHOTOCHEMICAL PATHS: THE PHOTOCHEMICAL AND PHOTOPHYSICAL LIMITS" @default.
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- W155389017 doi "https://doi.org/10.1016/b978-0-08-023942-2.50011-0" @default.
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