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- W1560631557 abstract "The computations performed in a previous paper for hypothetical structures of the site active in the polymerization of olefins at the (110) surfaces of TiCl3-α are extended to edges, steps and reliefs on (111) surfaces of all the layered modifications of TiCl3. Our computations suggest that edges, steps and reliefs of all the layered modifications of TiCl3 should behave similarly in providing active sites; polymerization should occur on these more exposed sites because of the much lower activation energies than for plain surfaces. A unique general model emerges: lower steric repulsions appear to be implied for a coordination of the polymeric chain on the more hindered octahedral position at a titanium atom and this, in turn, causes a chiral orientation of the first carbon-carbon bond of the chain. This orientation may be the main factor in determining the stereospecificity." @default.
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- W1560631557 date "1980-01-01" @default.
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- W1560631557 title "Analysis of models for the ziegler-natta stereospecific polymerization on the basis of non-bonded interactions at the catalytic site—II" @default.
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- W1560631557 doi "https://doi.org/10.1016/0014-3057(80)90113-5" @default.
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