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• W1562698619 endingPage "6297" @default.
• W1562698619 startingPage "6288" @default.
• W1562698619 abstract "We present a comprehensive experimental study of bound excited states in I−Xen clusters (n=1–54), using photoelectron spectroscopy and energy-dependent action spectroscopy. Starting at n=4, the electron detachment action spectra developed peaks lying in energy lower than the vertical binding energy. This behavior has been shown for both final spin states of the neutral iodine. It indicates the existence of bound electronic states extended over the xenon cluster. The peaks lying in energy below the J=1/2 detachment continuum of the iodine (n&gt;4) were detected over the whole cluster size range of I−Xen using electron detachment action spectroscopy. For the bound states relating to the J=3/2 continuum, in the size range n=4–12, thermionic emission has marked the existence of bound states. For n&gt;12, these states were stabilized and detected via two-photon excitations. The picture, unveiled from the above photoelectron and action spectra, is the gradual evolution of bound excited states on the xenon solvent cluster. The critical size for the binding of an excited electron is n=4. At the largest cluster interrogated, I−Xe54, the binding energy amounts to 170 meV. We compare these states to the ground electronic state of Xen− clusters, and discuss the differences between the experiments and model calculations." @default.
• W1562698619 created "2016-06-24" @default.
• W1562698619 creator A5041231739 @default.
• W1562698619 creator A5072344541 @default.
• W1562698619 date "1999-04-01" @default.
• W1562698619 modified "2023-10-16" @default.
• W1562698619 title "Photodetachment studies of extended excited states in I−Xen clusters (n=1–54)" @default.
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• W1562698619 doi "https://doi.org/10.1063/1.478533" @default.
• W1562698619 hasPublicationYear "1999" @default.
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