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- W1566239432 abstract "Publisher Summary This chapter predicts the various reaction products formed by exposing alloys to particular gases, and the effects of temperature and pressure on the outcome. This requires the use of chemical thermodynamics, and in particular, the use of phase equilibria. The rates at which the products form are usually governed by diffusion and interfacial processes, both involving crystallographic defects. Finally, the structural integrity of any solid is determined by its mechanical state. The chapter reviews these areas, focusing on their application to high temperature oxidation reactions. The thermodynamics of solutions can be derived from their enthalpy and entropy of mixing. An ideal solution is a completely random mixture of constituents, which experience the same thermal interaction with all neighboring atoms, and the entropy of mixing is purely configurational. In developing a more accurate description of diffusion, several approaches are possible. These include geometric, random walk procedures, which have been applied to crystalline solids to yield an advanced theory of correlation and isotope effects, and the application of absolute rate theory. In the most common diffusion measurements, the movement of a system towards homogeneity is observed and compared with the predictions of the diffusion equations. If sample dimensions and the period of diffusion are such that concentrations at the ends of the sample do not change, then the experiment is described as an infinite diffusion couple." @default.
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- W1566239432 date "2008-01-01" @default.
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- W1566239432 title "Chapter 2 Enabling Theory" @default.
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