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- W1566265596 abstract "A method for estimating vibrational quantum numbers of vibrationally excited transients in solution is proposed. In this method, we calculate anti-Stokes Raman excitation profiles (REPs) which are characteristic of the initial vibrational states involved in the Raman process, and compare them with observed anti-Stokes intensities. We have applied this method to vibrationally hot molecules of canthaxanthin in the S o state and those of trans-stilbene in the S 1 state. For canthaxanthin, it has been found that the vibrationally excited transients are for the most part on the ν=1 level of the C═C stretching mode, and that excess vibrational energy is statistically distributed among all intramolecular vibrational modes. As for S 1 stilbene, vibrational transients are shown to be mostly on the ν=1 level for two vibrational modes examined, while the excess vibrational energy is probably localised on the olefinic C═C stretching mode." @default.
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- W1566265596 date "1999-01-01" @default.
- W1566265596 modified "2023-10-17" @default.
- W1566265596 title "Picosecond Anti-Stokes Raman Excitation Profiles as a Method for Investigating Vibrationally Excited Transients" @default.
- W1566265596 doi "https://doi.org/10.1155/1999/21312" @default.
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