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- W1566445702 abstract "This chapter presents periodic mesoporous organosilicas. The synthesis of hybrid materials via hydrolysis and condensation reactions of bridged organosilsesquioxane precursors [(R’O)3Si-R-Si(OR’)3] have been known from the sol–gel chemistry for quite some time. In contrast to the organofunctionalized mesoporous silica the organic units in this kind of materials are two-point attached within the silica matrix through covalent bonds and thus homogenously distributed, being a genuine part of the 3D framework structure. Combining the two approaches, that is using the bridged polysilsesquioxane precursors known from the sol–gel chemistry and bringing them to reaction in the presence of the supramolecular aggregates of long-chain surfactants results in the formation of periodic mesoporous organosilicas (PMOs), in which the organic functionalities are not only completely homogeneously distributed but possess additionally ordered pore arrangements accompanied with sharp pore size distributions. An overview of the structures of the polysilsesquioxane precursors, which could successfully converted to PMO materials is presented." @default.
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- W1566445702 date "2008-01-01" @default.
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- W1566445702 title "Periodic mesoporous organosilicas (PMOs): a new class of materials is coming of age" @default.
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- W1566445702 doi "https://doi.org/10.1016/s0167-2991(08)80151-6" @default.
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