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- W1566707170 abstract "The role of a Pt/Al 2 O 3 catalyst in the oxidative dehydrogenation of light paraflins was investigated by means of a novel annular reactor which allows to realize very high space velocities and controlled temperature conditions. While a number of previous papers claimed that Pt is extremely active in the selective oxidation to olefins, the experiments in the annular reactor showed that the present noble-metal catalyst is highly active in the non selective oxidation to CO x , H 2 and H 2 0 only. Gas-phase experiments and simulations of a homogeneous reactor showed that the formation of olefins at high temperature and short contact times can be largely explained by the gas-phase oxidative pyrolysis. However, autothermal experiments demonstrated that the catalytic phase can be exploited in an adiabatic reactor for igniting and thermally supporting the pyrolytic process; the combined catalytic-homogeneous reactor performed as a homogeneous reactor, but the presence of the catalyst allowed to produce high yields to olefms at much lower reactor volume and lower pre-heat temperatures." @default.
- W1566707170 created "2016-06-24" @default.
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- W1566707170 date "2000-01-01" @default.
- W1566707170 modified "2023-09-27" @default.
- W1566707170 title "Experimental and theoretical investigation on the roles of heterogeneous and homogeneous phases in the oxidative dehydrogenation of light paraffins in novel short contact time reactors" @default.
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- W1566707170 doi "https://doi.org/10.1016/s0167-2991(00)80481-4" @default.
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