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- W1569703710 abstract "The neo-pentane hydrogenolysis turn-over frequency (TOF) of platinum on macroporous acidic SiO2-Al2O3 is about 500 times higher than that on basic MgO-Al2O3 hydrotalcite clay. The TOF increases with increasing electronegativity of the support oxygen ions similar to that found for Pt dispersed in microporous supports, such as LTL and Y zeolite. In addition, for Pt on silica-alumina, the intensity of the Fourier transform of the atomic XAFS oscillations, which were isolated from the XAFS spectra is larger and shifted to lower radius. A general model for the metal-support interaction is proposed, where a Coulomb attraction causes an increase in ionisation potential of the metal d-valence orbitals with increasing electronegativity (i.e. lower electron density) of the support oxygen ions." @default.
- W1569703710 created "2016-06-24" @default.
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- W1569703710 date "2000-01-01" @default.
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- W1569703710 title "An atomic XAFS study of the metal-support interaction in Pt/SiO2-Al2O3 and Pt/MgO-Al2O3 catalysts: an increase in ionisation potential of platinum with increasing electronegativity of the support oxygen ions" @default.
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- W1569703710 doi "https://doi.org/10.1016/s0167-2991(00)80976-3" @default.
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