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- W1569871361 abstract "Optical stimulation of surface reactions has attracted considerable attention, both as a test bed for probing fundamental chemical events and as an avenue for novel low temperature surface modification. The impact areas for the associated optically driven reactions range from materials synthesis and modification to environmental remediation. To optimally exploit lasers in these surface processes, it is essential to understand reaction and energy transfer pathways of adsorbates on surfaces. This project is directed at establishing the dominant energy transfer mechanisms in these reactions. The authors have focused their efforts on deposition systems where the relevant adsorbates are typically organometallic molecules. Ideally, the laser radiation will strip away the ligands, which desorb into the gas phase, leaving behind a pattered layer of metal atoms. In reality, there are a number of competing pathways, such as energy transfer and ligand interactions, which interfere with this ideal picture. To serve as a model system in the characterization of laser-induced deposition, the photodecomposition dynamics of Mo(CO){sub 6}/Si(111) 7x7 have been probed by applying surface sensitive diagnostics to follow the photomodified surface and state-selective detection techniques to establish the energy content of the evolved CO photoproduct." @default.
- W1569871361 created "2016-06-24" @default.
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- W1569871361 date "1994-07-01" @default.
- W1569871361 modified "2023-09-24" @default.
- W1569871361 title "Optically driven surface reactions: Laser probes of surface dynamics. Final report" @default.
- W1569871361 doi "https://doi.org/10.2172/10166720" @default.
- W1569871361 hasPublicationYear "1994" @default.
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