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• W1576136370 abstract "Electronic band structures of two novel semiconducting nitrides of the group‐IV elements of Th 3 P 4 ‐type crystal structure, c‐M 3 N 4 , where MZr or Hf, is investigated using an element specific soft X‐ray spectroscopy for the first time. From the pairs of N 1s X‐ray absorption and N 2p → 1s resonant X‐ray emission spectra partial densities of states (PDOS) of nitrogen, predicted to be strongly hybridized with those of the metals, are obtained for both compounds. From these data the electronic band gaps of oxygen bearing c‐Zr 3 N 4 and of c‐Hf 3 N 4 , predicted before to be direct or nearly direct, are derived to be E g = 1.6 eV and E g = 1.8 eV, respectively. While the experimentally determined E g for c‐Hf 3 N 4 agrees with the theoretical one obtained using the local density approximation (LDA) method, the E g measured for oxygen bearing c‐Zr 3 N 4 is significantly higher than those calculated using both the LDA and the generalized gradient approximation method. The examined compounds, having high hardness, elastic moduli and oxidation resistance, appear to be multifunctional materials suitable also for applications as (opto)electronic materials. Band gap evolution in c‐M 3 N 4 nitrides as a function of the cation type, Zr or Hf." @default.
• W1576136370 created "2016-06-24" @default.
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• W1576136370 date "2013-12-27" @default.
• W1576136370 modified "2023-09-30" @default.
• W1576136370 title "Electronic structure and band gap of oxygen bearing c-Zr₃ N₄ and of c-Hf₃ N₄ by soft X-ray spectroscopy" @default.
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• W1576136370 doi "https://doi.org/10.1002/pssa.201330338" @default.
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