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- W1581216731 abstract "Abstract : Combining the techniques of direct excitation of overtone vibrations and time resolved spectroscopic detection permits detailed measurements of the vibrational and rotational relaxation of highly vibrationally excited molecules. Using this technique, we have measured vibrational and rotational relaxation in HF(v=3,4,5,). By observing near-infrared fluorescence, we determine the self-relaxation probabilities for HF(v=3,4,5) to be 0.19, 0.47, and 0.97, respectively, and find that the rates decrease more rapidly with temperature in these high levels than for v=1. Using laser double resonance to probe individual rotational states, we find phenomenological rotational relaxation rate constants which decrease montonically with rotational energy change in the vibrationally excited molecule. (Author)" @default.
- W1581216731 created "2016-06-24" @default.
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- W1581216731 date "1981-03-01" @default.
- W1581216731 modified "2023-09-22" @default.
- W1581216731 title "Collisional Energy Transfer in Highly Vibrationally Excited Molecules." @default.
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