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- W1581248192 abstract "Soft X-ray absorption fine structure (SOXAFS) studies of the aluminium K edge have been used to study the local structure around aluminium in the zeolites Na-FAU and H-ZSM-5. As expected, the local enviroment in Na-FAU is symmetric, consisting of four oxygen atoms arranged in a regular tetrahedron, at distance of 1.74from aluminium. In the acidic H-ZSM-5, (Si/Al ratio 18) this tetrahedron is no longer symmetric. One Al-O distance is lengthened to 1.98 , and this is identified as that involving the acidic Al-O(H)-Si entity. Changes in the Al-O Al angles allow conclusions to be drawn on how the zeolite structure adjusts to the presence of the acidic moieties. The result support theoretical predictions for this material, and are shown to be highly consistent numerically with the averaged information provided by previous X-ray diffraction studies." @default.
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- W1581248192 date "2004-01-01" @default.
- W1581248192 modified "2023-09-23" @default.
- W1581248192 title "A soft X-ray exafs study of the local structure of tetrahedral aluminium in zeolites" @default.
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- W1581248192 doi "https://doi.org/10.1016/s0167-2991(04)80657-8" @default.
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