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- W1583942739 abstract "Carbon nitride polymers were prepared for the first time by the pyrolysis of 3,5-disubstituted-1,2,4-triazole derivatives, namely, 3,5-diamino-1,2,4-triazole [1] and 3-amino-1,2,4-triazole-5-thiol [2], in bulk as well as in LiCl/KCl salt melts. The reaction of [1] and [2] in bulk yields condensed heptazine-based polymers, while in LiCl/KCl eutectics it leads to the formation of well-defined potassium poly(heptazine imides), according to the results of 13C NMR and XPS investigations, whose formation resembles that of emeraldine salts of polyaniline. The density functional calculations supported the structural model suggested for potassium poly(heptazine imide) polymer. Owing to the specific reaction path, the products obtained from triazoles therefore show electronic properties rather different to known carbon nitrides, such as band gap and conduction and valence bands positions. With the degree of crystallinity of the reference materials, triazole-derived carbon nitrides are characterized by almost comple..." @default.
- W1583942739 created "2016-06-24" @default.
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- W1583942739 date "2015-07-24" @default.
- W1583942739 modified "2023-10-13" @default.
- W1583942739 title "Triazoles: A New Class of Precursors for the Synthesis of Negatively Charged Carbon Nitride Derivatives" @default.
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- W1583942739 doi "https://doi.org/10.1021/acs.chemmater.5b00812" @default.
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