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- W1585846209 abstract "We report on structures, magnetisms, and transport properties of two new barium ruthenates, 10H-type BaRuO3 and Ba2Ru7O18. The crystal structure of 10H-BaRuO3 consists of face-shared dimers and trimers of RuO6 octahedra. The magnetic susceptibility of 10H-BaRuO3 is 7.7×10−4 emu/mol at RT. We interpret its very weak temperature dependence as Pauli paramagnetism enhanced by electron correlations. The resistivity of 10H-BaRuO3 is 8.5×10−2 Ω cm at 296 K. The slope of the R versus T curve is negative in the whole temperature. It indicates metallic or semi-metallic electronic states. The structure of Ba2Ru7O18 is composed of edge-shared trimers and tetramers of RuO6 octahedra. The magnetic susceptibility of Ba2Ru7O18 is 3.7×10−4 emu/mol Ru at RT. Its almost temperature-independent character is also explained in terms of Pauli paramagnetism enhanced by electron correlations. The resistivity of Ba2Ru7O18 is 6.7×10−4 Ω cm at 296 K. In this case, the slope of the R versus T curve is positive, and the temperature dependence is linear to T1.2 below 25 K. This shows a large deviation from a Fermi-liquid criterion." @default.
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- W1585846209 date "2004-11-01" @default.
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- W1585846209 title "New ternary barium ruthenates: 10H-type BaRuO3 and Ba2Ru7O18" @default.
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- W1585846209 doi "https://doi.org/10.1016/j.jallcom.2004.04.035" @default.
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