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• W1585938862 abstract "A greatly-improved voltaic cell, based on the Kenrick cell and using a mercury jet reference electrode, has been made and tested. The cell is capable of measuring a compensating potential difference (cpd) to =0.1 mV or better, a precision comparable with that obtainable with well-behaved galvanic cells. The cpd's of the cells: Hg(N2)||HCl(aq, m)|Pt, H2 Hg(N2)||HCl(aq, m)|AgCl|Ag have been measured for 0.001<m/mol kg−1<0.5 at 298 K. For 0.001<m/mol kg−1<0.02, the solution surface potential drops rapidly by ca. 5 mV, before beginning to rise steadily with increasing HCl concentration. The low concentration drop in surface potential is interpreted as evidence for the penetration by ions of the permanent dipole layer at the solution-gas interface. A previously-proposed electrostatic model describing this phenomenon accounts quantitatively for the observed changes in the solution surface potential (Xm) at low concentrations. The model provides a theoretical basis for a function from which a standard state cpd (Ec0) can be determined by extrapolation to infinite dilution. On the basis of this analysis, we estimate the surface potential of pure water (X0) to be 25±10 mV at 298 K." @default.
• W1585938862 created "2016-06-24" @default.
• W1585938862 creator A5016161458 @default.
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• W1585938862 date "1982-10-01" @default.
• W1585938862 modified "2023-10-10" @default.
• W1585938862 title "Precise compensating potential difference measurements with a voltaic cell" @default.
• W1585938862 cites W1968003297 @default.
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• W1585938862 doi "https://doi.org/10.1016/0022-0728(82)85102-4" @default.
• W1585938862 hasPublicationYear "1982" @default.
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