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- W1589610679 abstract "In order to attempt a quantitative analysis of voltammograms of hydrogen adsorption on platinum surfaces in sulphuric acid medium, a numerical deconvolution by choosing an adsorption isotherm was carried out. The principle of this deconvolution and the choice of the isotherm to be used, the Frumkin-Fowler isotherm, was discussed in Part I and applied first to several voltammograms of various initial states of Pt(100). In the second part, deconvolutions of voltammograms of Pt(110), of three stepped surfaces, Pt(511), Pt(310) and Pt(21), and of the polyoriented surface of the spherical platinum single crystal are given. It is shown that the observation on the voltammogram of stepped surfaces of adsorption states common to those of basal surfaces depends on the size of the ordered domain of basal symmetry. The potential position and population of the various adsorption states of most of the stepped surfaces are in good agreement with the terrace-step model and confirm the assumption that they help in characterization of the symmetry of the adsorption sites and their surface arrangement. The voltammogram of the polyoriented surface is interprted with the help of the deconvolution of two oriented surfaces, Pt (100) and Pt (110). Each of the six states of this surface obtained after deconvolution between 0.075 and 0.375 V (vs. RHE) is ascribed to a hydrogen adsorption state on a (100) or (110) site." @default.
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- W1589610679 date "1987-09-01" @default.
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- W1589610679 title "Quantitative analysis of the distribution of the hydrogen adsorption states at platinum surfaces" @default.
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- W1589610679 doi "https://doi.org/10.1016/0022-0728(87)85020-9" @default.
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