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• W1590294080 endingPage "254001" @default.
• W1590294080 startingPage "254001" @default.
• W1590294080 abstract "The ionic conduction and electrochemical and thermal stabilities of the LiBH4-LiCl solid-state electrolyte were investigated for use in bulk-type all-solid-state lithium-sulfur batteries. The LiBH4-LiCl solid-state electrolyte exhibiting a lithium ionic conductivity of [Formula: see text] at 373 K, forms a reversible interface with a lithium metal electrode and has a wide electrochemical potential window up to 5 V. By means of the high-energy mechanical ball-milling technique, we prepared a composite powder consisting of elemental sulfur and mixed conductive additive, i.e., Ketjen black and Maxsorb. In that composite powder, homogeneous dispersion of the materials is achieved on a nanometer scale, and thereby a high concentration of the interface among them is induced. Such nanometer-scale dispersals of both elemental sulfur and carbon materials play an important role in enhancing the electrochemical reaction of elemental sulfur. The highly deformable LiBH4-LiCl electrolyte assists in the formation of a high concentration of tight interfaces with the sulfur-carbon composite powder. The LiBH4-LiCl electrolyte also allows the formation of the interface between the positive electrode and the electrolyte layers, and thus the Li-ion transport paths are established at that interface. As a result, our battery exhibits high discharge capacities of 1377, 856, and 636 mAh g(-1) for the 1st, 2nd, and 5th discharges, respectively, at 373 K. These results imply that complex hydride-based solid-state electrolytes that contain Cl-ions in the crystal would be integrated into rechargeable batteries." @default.
• W1590294080 created "2016-06-24" @default.
• W1590294080 creator A5007227263 @default.
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• W1590294080 date "2015-06-04" @default.
• W1590294080 modified "2023-10-18" @default.
• W1590294080 title "Pseudo-binary electrolyte, LiBH₄–LiCl, for bulk-type all-solid-state lithium-sulfur battery" @default.
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• W1590294080 doi "https://doi.org/10.1088/0957-4484/26/25/254001" @default.
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• W1590294080 hasPublicationYear "2015" @default.
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