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• W1593302941 abstract "The influence of higher-order terms in the Barker–Henderson approximation to the Zwanzig perturbation expansion is examined for a Lennard-Jones fluid. We find that the error introduced by ignoring these higher-order terms is negligible compared with the error due to the replacement of the reference system by a hard-sphere system in which the diameter of the spheres ensures coincidence to only first order between the free energy of the reference system and the free energy of the hard-sphere system. In calculating the contribution to the pressure due to the perturbation, one often uses the Percus–Yevick solution for the hard-sphere reference system. The error introduced by this approximation is found to be considerable." @default.
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• W1593302941 date "1970-09-15" @default.
• W1593302941 modified "2023-09-25" @default.
• W1593302941 title "Equation of State for a Lennard‐Jones Fluid" @default.
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• W1593302941 doi "https://doi.org/10.1063/1.1674336" @default.
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