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- W1597112846 abstract "This chapter focuses on two processes of relevance to corrosion: surface mobility, enhanced by an electric field or by co-adsorbed chlorine atoms, and hydrogen evolution on pure metals and nanostructures. It discusses the principles that underlie the kinetic Monte Carlo (KMC) method, and the way the inputs for the simulation were obtained. It also discusses the effect of an electric field on electrodes of silver, and describes step fluctuations and the analysis of island shapes. The combination of large-scale KMC simulations with density functional theory (DFT) calculations and analytically solvable thermodynamic models yield a good agreement with experiments on two-dimensional Ostwald ripening on Ag and Au metals in a bare fcc surface or in chlorine containing electrolytes. The chapter presents a theory of electrochemical reactions, in which charge is transferred through the interface, and the electrode potential affects directly the free energy of the reaction." @default.
- W1597112846 created "2016-06-24" @default.
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- W1597112846 date "2015-04-21" @default.
- W1597112846 modified "2023-10-13" @default.
- W1597112846 title "Processes at Metal–Solution Interfaces" @default.
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- W1597112846 doi "https://doi.org/10.1002/9781119057666.ch3" @default.
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