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- W1597624056 abstract "A time resolved resonance Raman (TR 3 ) study of 1-nitronaphthalene (1NN) first triplet excited state in various solvents is combined with ab initio calculations to determine the nature and the geometry of this state in environments of different polarity. A transient absorption and TR 3 study of the reactions of triplet 1NN with trans-stilbene (tS) in solution in both non-polar and polar solvents is reported. In polar solution, 3 1NN acts as an electron acceptor whereas in non-polar solution only energy transfer to tS is observed. Moreover, at high concentrations of tS, the radical cation tS + reacts with ground-state tS to form a dimer radical cation (tS 2 ) + . Differences between the Raman spectra of the monomeric and the dimeric radical cations are reported in the 1500–1650 cm -1 region. The switch from energy to electron transfer when going from nonpolar to polar solutions is discussed in terms of the Marcus-Hush theory of electron transfer." @default.
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- W1597624056 date "1999-01-01" @default.
- W1597624056 modified "2023-09-27" @default.
- W1597624056 title "Triplet 1-Nitronaphthalene and Competitive Energy and Electron Transfer Reactions With Trans-Stilbene" @default.
- W1597624056 doi "https://doi.org/10.1155/1999/92415" @default.
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