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- W1597742283 abstract "Copper exchanged MCM-22 zeolites with varying copper contents were prepared, characterized and tested in the nitrous oxide decomposition. Over-exchanged samples showed high activity, comparable to very active Cu-ZSM-5 catalysts. The nature of the copper species was investigated by TPR-H 2 , FTIR-CO and FTIR-NO, evidencing at least three different species: exchanged Cu 2+ ions, cationic oligomeric species and oxidic phases. Upon NO adsorption, mononitrosilic complexes Cu I -(NO) were formed, and completely oxidized to Cu II -(NO) with increasing NO pressure. Nitrate complexes were extensively formed by reaction with the oxidic phases in the sample with 183% cation exchange level." @default.
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- W1597742283 date "2002-01-01" @default.
- W1597742283 modified "2023-09-26" @default.
- W1597742283 title "Spectroscopic and catalytic studies on Cu-MCM-22: Effect of copper loading" @default.
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- W1597742283 doi "https://doi.org/10.1016/s0167-2991(02)80047-7" @default.
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