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- W1598867897 abstract "The vapour phase synthesis of ethylbenzene from 1,3-butadiene was investigated using FAU-type zeolites with basic properties. The influence of basicity was studied by: (1) variation of the Si/Al-ratio, (2) ion-exchange with cesium and (3) impregnation with sodium or cesium salts. One-step direct aromatization of 1,3-butadiene is possible by using these zeolites as bifunctional Lewis-acid/base catalysts but suffers from strong deactivation. Consequently the reaction should be performed in two separate steps. For the second reaction step—the vapour phase conversion of 4-vinylcyclohexene (which can be easily synthesized from 1,3-butadiene) to ethylbenzene—basic zeolites represent useful catalysts, especially those obtained by impregnation with alkali metal salts. Applying molecular modelling techniques to study the sorption at reaction conditions was (in combination with experiments) very helpful to demonstrate that deactivation results from product inhibition." @default.
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- W1598867897 date "2000-01-01" @default.
- W1598867897 modified "2023-10-18" @default.
- W1598867897 title "Synthesis of ethylbenzene from 1,3-butadiene using basic zeolite catalysts" @default.
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- W1598867897 doi "https://doi.org/10.1016/s0167-2991(00)81067-8" @default.
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