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- W1600914675 abstract "A general picture of the mechanism of oxidative methane coupling over metal oxides has been proposed on the basis of kinetic and CH4-CD4 exchange studies on Sm2O3. The rate-determining step is the hydrogen abstraction from the methane activated on the surface. A diatomic oxygen species, probably O2 2−, is responsible for the abstraction of hydrogen. This active oxygen must be in equilibrium with the gaseous oxygen. Lattice oxygen atoms do not contribute to the oxidative coupling reaction. The main products in the ethanes formed in the reaction of the mixture of CH4, CD4, and O2 were CH3CH3, CH3CD3, and CD3CD3, indicating that the CH3. radical in the gas phase or the CH3 group on the surface is the reaction intermediate." @default.
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- W1600914675 date "1992-01-01" @default.
- W1600914675 modified "2023-09-23" @default.
- W1600914675 title "Partial Oxidation of Methane over Metal Oxides: Reaction Mechanism and Active Oxygen Species" @default.
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- W1600914675 doi "https://doi.org/10.1007/978-94-015-7449-5_3" @default.
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