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• W1601144637 abstract "The stochastic thermodynamics of a dilute, well-stirred mixture of chemically reacting species is built on the stochastic trajectories of reaction events obtained from the chemical master equation. However, when the molecular populations are large, the discrete chemical master equation can be approximated with a continuous diffusion process, like the chemical Langevin equation or low noise approximation. In this paper, we investigate to what extent these diffusion approximations inherit the stochastic thermodynamics of the chemical master equation. We find that a stochastic-thermodynamic description is only valid at a detailed-balanced, equilibrium steady state. Away from equilibrium, where there is no consistent stochastic thermodynamics, we show that one can still use the diffusive solutions to approximate the underlying thermodynamics of the chemical master equation." @default.
• W1601144637 created "2016-06-24" @default.
• W1601144637 creator A5067805186 @default.
• W1601144637 date "2015-07-28" @default.
• W1601144637 modified "2023-09-27" @default.
• W1601144637 title "Diffusion approximations to the chemical master equation only have a consistent stochastic thermodynamics at chemical equilibrium" @default.
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• W1601144637 doi "https://doi.org/10.1063/1.4927395" @default.
• W1601144637 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26233111" @default.
• W1601144637 hasPublicationYear "2015" @default.
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