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- W1601845896 abstract "We present a nonperturbative time-dependent quantum mechanical theory of the laser catalysis and control of a bifurcating A+BC↔ℏω0ABC*(v)↔ℏω0AB+C reaction, with ABC*(v) denoting an intermediate, electronically excited, complex of ABC in the vth vibrational state. We apply this theory to the low collision energy fermion-boson light-induced exchange reaction, Li6(S2)+Li27(Σu+3)↔ℏω0(Li6Li7Li7)*↔ℏω0Li6Li7(Σ+3)+Li7(S2). We show that at very low collision energies and energetically narrow (∼0.01cm−1) initial reactant wave packets, it is possible to tune the yield of the exchange reaction from 0 to near-unity (yield ⩾99%) values. Controllability is somewhat reduced at collisions involving energetically wider (∼1cm−1) initial reactant wave packets. At these energetic bandwidths, the radiative reactive control, although still impressive, is limited to the 0%–76% reactive-probabilities range." @default.
- W1601845896 created "2016-06-24" @default.
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- W1601845896 date "2008-03-28" @default.
- W1601845896 modified "2023-09-27" @default.
- W1601845896 title "Theory of laser enhancement and suppression of cold reactions: The fermion-boson Li6+Li27↔ℏω0Li6Li7+Li7 radiative collision" @default.
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- W1601845896 doi "https://doi.org/10.1063/1.2899666" @default.
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