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• W1605213202 endingPage "1026" @default.
• W1605213202 startingPage "1024" @default.
• W1605213202 abstract "Past efforts to achieve selective bond scission by vibrational excitation have been thwarted by energy thermalization. Here we report resonant photodesorption of hydrogen from a Si(111) surface using tunable infrared radiation. The wavelength dependence of the desorption yield peaks at 0.26 electron volt: the energy of the Si-H vibrational stretch mode. The desorption yield is quadratic in the infrared intensity. A strong H/D isotope effect rules out thermal desorption mechanisms, and electronic effects are not applicable in this low-energy regime. A molecular mechanism accounting for the desorption event remains elusive." @default.
• W1605213202 created "2016-06-24" @default.
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• W1605213202 date "2006-05-19" @default.
• W1605213202 modified "2023-09-25" @default.
• W1605213202 title "Desorption of H from Si(111) by Resonant Excitation of the Si-H Vibrational Stretch Mode" @default.
• W1605213202 cites W1987869326 @default.
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• W1605213202 doi "https://doi.org/10.1126/science.1124529" @default.
• W1605213202 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16709778" @default.
• W1605213202 hasPublicationYear "2006" @default.
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