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• W1605643265 abstract "The electrochemical reduction of CO2 has been studied on differently prepared Cu electrodes. The effect of electrode treatment on current efficiency (CE) for the formation of CO2 reduction products and duration of the electrode catalytic activity under specified electrolysis conditions were studied. Significant performance differences were found between rough and smooth surface electrodes and between thermally and non-thermally treated electrodes. A rough surface was much more active than a smooth one in terms of CE and catalytic electrode life. The total CE for hydrocarbon production (CH4, C2H4) increased with electrolysis time during the first electrolysis stage and decreased afterwards. For the formation of CH4 a two-path reaction scheme was proposed. The electrode deactivation was attributed to the formation of a poisonous intermediate, which is the same both for the CH2O and CO2 reduction. Experiments were performed at 25°C under atmospheric CO2 pressure in 0.5 M KHCO3 solution." @default.
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• W1605643265 date "1992-01-01" @default.
• W1605643265 modified "2023-09-30" @default.
• W1605643265 title "Electroreduction of CO2 on differently prepared copper electrodes" @default.
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• W1605643265 doi "https://doi.org/10.1016/0022-0728(92)80079-j" @default.
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