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• W1607952031 abstract "Assessment of the impacts of brown carbon (BrC) requires accurate determination of its physical properties, but a model must be invoked to derive these from instrument data. Ambient measurements were made in London at a site influenced by traffic and solid fuel (principally wood) burning, apportioned by single particle soot photometer data and optical properties measured using multiwavelength photoacoustic spectroscopy. Two models were applied: a commonly used Mie model treating the particles as single-coated spheres and a Rayleigh-Debye-Gans approximation treating them as aggregates of smaller-coated monomers. The derived solid fuel BrC parameters at 405 nm were found to be highly sensitive to the model treatment, with a mass absorption cross section ranging from 0.47 to 1.81 m2/g and imaginary refractive index from 0.013 to 0.062. This demonstrates that a detailed knowledge of particle morphology must be obtained and invoked to accurately parameterize BrC properties based on aerosol phase measurements." @default.
• W1607952031 created "2016-06-24" @default.
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• W1607952031 date "2015-01-23" @default.
• W1607952031 modified "2023-10-12" @default.
• W1607952031 title "The effect of complex black carbon microphysics on the determination of the optical properties of brown carbon" @default.
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• W1607952031 doi "https://doi.org/10.1002/2014gl062443" @default.
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