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- W1609826620 abstract "The experimental determination of solid state electronic band structure was shown to be feasible through angle resolved photoelectron spectroscopic (ARPES) studies of the valence bands of oriented copper single crystals. In order to assign features observed in ARPES spectra to solid state energy bands, the theoretical description of the photoemission process must be understood in detail. For this purpose, the influence of the excitation process, hot electron transport, and surface effects on observed spectra are considered carefully. First, photoemission from atomic neon is examined theoretically to learn the nature of the continuum final state and its relation to the total and differential atomic cross sections. The directionality of the band-like final states in a crystalline solid is then determined by examining ARPES spectra collected from Cu single crystals. Inelastic scattering processes in a solid cause attenuation of photocurrent, which is studied by studying the surface sensitivity of plasmon loss satellites in photoemission spectra of Al and In. The effect of photocurrent damping on ARPES valence band spectra of copper is then investigated by examining the relaxation of crystal momentum selection rules with increased surface sensitivity. The presence of the surface itself is important in determining angular distributions, as shown by measurements of photoelectron refraction. Photoemission is also possible from states localized at the surface, and examples of surface state photoemission are found from the (111) and (211) surfaces of copper. Finally, the dynamic effects of thermal lattice disordering are shown to be extremely important in photoemission studies applied to band structure determinations, as electron-phonon interactions can suppress the information content of an ARPES spectrum drastically." @default.
- W1609826620 created "2016-06-24" @default.
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- W1609826620 date "1978-05-01" @default.
- W1609826620 modified "2023-09-23" @default.
- W1609826620 title "Angle-resolved photoelectron spectroscopy applied to the determination of the surface electronic structure of crystalline metals" @default.
- W1609826620 doi "https://doi.org/10.2172/6762579" @default.
- W1609826620 hasPublicationYear "1978" @default.
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