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• W1611641119 endingPage "1230" @default.
• W1611641119 startingPage "1223" @default.
• W1611641119 abstract "The photodissociation of CH2XCH2Y (X,Y=Br,Cl) through absorption of 193 nm photons was investigated using product translational spectroscopy. No stable CH2BrCH2 or CH2ClCH2 was detected. The recorded time-of-flight spectra indicate that these internally excited radicals dissociated into Y+C2H4 in a concerted reaction with the first C–X bond rupture. Product anisotropy implies that the overall reaction time for three-body formation is in a fraction of rotational period. According to an asynchronous concerted reaction model, the measured spectra were simulated with product translational energy distributions coupled by asymmetric angular distributions. For the mixed halide, CH2BrCH2Cl, triple products Br+Cl+C2H4 can be originated from the cleavage of either the C–Br bond or the C–Cl bond. The results are discussed and where appropriate, comparisons with previous investigations of the related molecules are included." @default.
• W1611641119 created "2016-06-24" @default.
• W1611641119 creator A5018946567 @default.
• W1611641119 creator A5068347628 @default.
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• W1611641119 date "2004-01-13" @default.
• W1611641119 modified "2023-09-23" @default.
• W1611641119 title "A concerted three-body formation X+Y+C2H4 in the photodissociation of CH2XCH2Y (X,Y=Br,Cl) at 193 nm" @default.
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• W1611641119 doi "https://doi.org/10.1063/1.1633262" @default.
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• W1611641119 hasPublicationYear "2004" @default.
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