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- W1613339968 abstract "The square of the electronic–vibrational transition moment for the (2,0) band of the cyano radical (CN), A 2Π←X 2Σ+, red system at 789.5 nm has been determined using a direct time-resolved absorption technique. The line strength of the R1(8.5) transition of 12C14N was measured by comparison to the known line strength of the H12C14N(001)←(000) P(8) infrared υ3 fundamental transition near 3.05 μm. The CN radical was created by pulsed-laser photolysis of cyanogen, (CN)2, in a mixture of H2 and (CN)2 in either Ar or He carrier gas at 293 K. Both CN and HCN were monitored by time-resolved absorption spectroscopy during the same photolysis laser pulse. A simple kinetic model was used to relate the two absorption features to each other. The square of the electronic–vibrational transition moment for the A←X(2,0) band was found to be 7.8±1.0×10−38 esu2 cm2 in good agreement with theoretical calculations based on ab initio quantum chemistry methods." @default.
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- W1613339968 date "1998-10-15" @default.
- W1613339968 modified "2023-09-28" @default.
- W1613339968 title "Experimental measurement of the transition moment for the (2,0) band of the CN A 2Π←X 2Σ+ red system at 789.5 nm" @default.
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- W1613339968 doi "https://doi.org/10.1063/1.477273" @default.
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