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• W1617285217 abstract "We investigate the thermodynamic and transport properties of molybdenum-doped BaFe${}_{2}$As${}_{2}$ (122) crystals, the first report of hole doping using a 4$d$ element. The chemical substitution of Mo in place of Fe is possible up to ensuremath{sim} 7$%$. For Ba(Fe${}_{1ensuremath{-}x}$Mo${}_{x}$)${}_{2}$As${}_{2}$, the suppression rate of the magnetic transition temperature with $x$ is the same as in 3$d$ Cr-doped 122 and is independent of the unit cell changes. This illustrates that the temperature-composition phase diagram for hole-doped 122 can be simply parameterized by $x$, similar to the electron-doped 122 systems found in the literature. Compared to 122 with a coupled antiferromagnetic order (${T}_{N}$) and orthorhombic structural transition (${T}_{0}$) at ensuremath{approx}132 K, 1.3$%$ Mo-doped 122 ($x=0.013$) gives ${T}_{N}={T}_{0}=125(1)$ K according to neutron diffraction results and features in specific heat, magnetic susceptibility, and electrical resistivity. The cell volume expands by ensuremath{sim}1$%$ with maximum Mo doping and ${T}_{N}$ is reduced to ensuremath{approx}90 K. There is a ${T}^{*}$ feature that is identified for lightly Cr- or Mo-doped 122 crystals, which is $x$ dependent. This low-temperature transition may be a trace of superconductivity." @default.
• W1617285217 created "2016-06-24" @default.
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• W1617285217 date "2012-01-03" @default.
• W1617285217 modified "2023-10-16" @default.
• W1617285217 title "Effect of molybdenum<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mn>4</mml:mn><mml:mi>d</mml:mi></mml:mrow></mml:math>hole substitution in BaFe<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>2</mml:mn></mml:msub></mml:math>As<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>2</mml:mn></mml:msub></mml:math>" @default.
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• W1617285217 doi "https://doi.org/10.1103/physrevb.85.024503" @default.
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