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• W1618802802 abstract "Spectroscopic techniques that aim to resolve the electronic configuration and local coordination of a central atom by detecting inner‐shell radiative decays following photoexcitation using hard X‐rays are presented. The experimental setup requires an X‐ray spectrometer based on perfect crystal Bragg optics. The possibilities arising from non‐resonant (X‐Ray Emission Spectroscopy — XES) and resonant excitation (Resonant Inelastic X‐Ray Scattering Spectroscopy — RIXSS, High‐Energy‐Resolution Fluorescence Detected (HERFD) XAS) are discussed when the instrumental energy broadenings of the primary (beamline) monochromator and the crystal spectrometer for x‐ray emission detection are on the order of the core hole lifetimes of the intermediate and final electronic states. The small energy bandwidth in the emission detection yields line‐sharpened absorption features. In transition metal compounds, electron‐electron interactions as well as orbital splittings and fractional population can be revealed. Combination with EXAFS spectroscopy enables to extent the k‐range beyond unwanted absorption edges in the sample that limit the EXAFS range in conventional absorption spectroscopy." @default.
• W1618802802 created "2016-06-24" @default.
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• W1618802802 date "2007-01-01" @default.
• W1618802802 modified "2023-09-24" @default.
• W1618802802 title "Hard X-Ray Photon-In-Photon-Out Spectroscopy with Lifetime Resolution — of XAS, XES, RIXSS and HERFD" @default.
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• W1618802802 doi "https://doi.org/10.1063/1.2436402" @default.
• W1618802802 hasPublicationYear "2007" @default.
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