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• W1620803553 abstract "We show how to achieve optical, spin-selective transitions from the ground state to excited orbital states of group-V donors (P, As, Sb, and Bi) in silicon. We consider two approaches based on either resonant, far-infrared (IR) transitions of the neutral donor or resonant, near-IR excitonic transitions. For far-IR light, we calculate the dipole matrix elements between the valley-orbit and spin-orbit split states for all the group-V donors using effective mass theory. We then calculate the maximum rate and amount of electron-nuclear spin-polarization achievable through optical pumping with circularly polarized light. We find this approach is most promising for Bi donors due to their large spin-orbit and valley-orbit interactions. Using near-IR light, spin-selective excitation is possible for all the donors by driving a two-photon $mathrm{ensuremath{Lambda}}$ transition from the ground state to higher orbitals with even parity. We show that externally applied electric fields or strain allow similar, spin-selective $mathrm{ensuremath{Lambda}}$ transition to odd-parity excited states. We anticipate these results will be useful for future spectroscopic investigations of donors, quantum control and state preparation of donor spin qubits, and for developing a coherent interface between donor spin qubits and single photons." @default.
• W1620803553 created "2016-06-24" @default.
• W1620803553 creator A5013674722 @default.
• W1620803553 creator A5018642214 @default.
• W1620803553 date "2015-11-11" @default.
• W1620803553 modified "2023-10-06" @default.
• W1620803553 title "Optical control of donor spin qubits in silicon" @default.
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• W1620803553 doi "https://doi.org/10.1103/physrevb.92.195411" @default.
• W1620803553 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5259753" @default.
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• W1620803553 hasPublicationYear "2015" @default.
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