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- W16234974 abstract "Abstract For alumina-supported PtRe, the deuterium exchange of cyclopentane at 100°C and low pressure is insensitive to bimetallic interaction, while hydrogenolysis of the same molecule at 240°C and 1 atm is specific for bimetallic cluster formation. For silica-supported samples, XRD confirmed that alloy formation is related to high selectivity for hydrogenolysis to methane. For PtRe/Y-Zeolite catalysts, and corresponding monometallics, Pt was ion exchanged into the zeolite and Re was introduced either via ion exchange using [Re(en)2O2]Cl (en=ethylenediamine), or via impregnation using NH4ReO4. TPR studies revealed that the reduction of the Re is catalyzed by the Pt in both cases. The hydrogenolysis of n-heptane suggests that under severe conditions PtRe clusters are formed even in physical mixtures of Pt/NaY and Re/NaY." @default.
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- W16234974 date "1988-01-01" @default.
- W16234974 modified "2023-09-27" @default.
- W16234974 title "Catalytic Evidence For the Formation of Mixed Metal Ensembles in Supported Ptre Catalysts" @default.
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- W16234974 doi "https://doi.org/10.1016/s0167-2991(09)60637-6" @default.
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