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- W1636699586 abstract "Evaluating the feasibility of CO2 geologic sequestration requires intensive numerical simulations of multiphase fluid flow. Such simulations involve the calculation of P-T-X data for mixtures of CO2, H2O and various salts as a function of temperature, pressure and salinity. A numerically efficient thermodynamic model was developed previously [1] for phase partitioning without salt effects, and was shown to provide an excellent match to experimental data in the range 12–100°C and up to 600 bar. Here, the model is extended to NaCl and CaCl2 solutions by including activity coefficients for aqueous CO2 derived from several literature sources. Two of these sources [2,3] yield the best results. The approach allows computing mutual solubilities in a noniterative manner with an accuracy typically within experimental uncertainty for solutions up to 6 molal NaCl and 4 molal CaCl2 (Figure 1). Figure 1. Measured (symbols) versus predicted (lines) CO2 solubilities using five different activity coefficient models." @default.
- W1636699586 created "2016-06-24" @default.
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- W1636699586 date "2004-07-24" @default.
- W1636699586 modified "2023-09-27" @default.
- W1636699586 title "A non-iterative model for H2O-CO2 mutual solubility in chloridebrines" @default.
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