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- W1640033178 abstract "The phenomenon of the decrease in the accelerating action of multicharged cations on the electroreduction of anions with increasing negative charge on the mercury electrode and with increasing concentration of KCl is investigated for inorganic cations of different size (K+, Ba2+, Ca2+, La3+, Lu3+, Y3+). This decrease for the electroreduction of anions of the first group is explained within the framework of the slow discharge theory in combination with the diffuse-layer model, considering the existence of two planes of the closest approach of cations and anions to the electrode surface and the decrease of the dielectric constant in the space between these planes compared with its value in the bulk solution. The ψ1 potentials at the center of the activated complex are calculated for different solution compositions in the presence of multicharged cations. This gives an opportunity to construct the corrected Tafel plots with the corresponding ψ1 potentials. It is shown that the effect of M3+ cations on the electroreduction of anions of the second group is connected with donor properties of water molecules in the hydrated spheres of these cations." @default.
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- W1640033178 date "1989-03-01" @default.
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- W1640033178 title "Ion size effects in the Hurwitz-Parsons analysis" @default.
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- W1640033178 doi "https://doi.org/10.1016/0022-0728(89)87155-4" @default.
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